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      Analysis of the Characteristics and Sources of Carbonaceous Aerosols in PM 2.5 in the Beijing, Tianjin, and Langfang Region, China

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          Abstract

          PM 2.5 samples from Beijing, Tianjin, and Langfang were simultaneously collected from 20 November 2016 to 25 December 2016, and the organic carbon (OC) and elemental carbon (EC) content in the samples were measured and analyzed. The pollution characteristics and sources of OC and EC in atmospheric PM 2.5 for three adjacent cities were discussed. The average mass concentrations of OC in PM 2.5 in Beijing, Tianjin, and Langfang were 27.93 ± 23.35 μg/m 3, 25.27 ± 12.43 μg/m 3, and 52.75 ± 37.97 μg/m 3, respectively, and the mean mass concentrations of EC were 6.61 ± 5.13 μg/m 3, 6.14 ± 2.84 μg/m 3, and 12.06 ± 6.81 μg/m 3, respectively. The average mass concentration of total carbon (TC) accounted for 30.5%, 24.8%, and 49% of the average mass concentration of PM 2.5 in the atmosphere. The total carbonaceous matter (TCA) in Beijing, Tianjin, and Langfang was 51.29, 46.57, and 96.45 μg/m 3, respectively. The TCA was the main component of PM 2.5 in the region. The correlation between OC and EC in the three cities showed R 2 values of 0.882, 0.633, and 0.784 for Beijing, Tianjin, and Langfang, respectively, indicating that the sources of urban carbonaceous aerosols had good consistency and stability. The OC/EC values of the three sampling points were 4.48 ± 1.45, 4.42 ± 1.77, and 4.22 ± 1.29, respectively, considerably greater than 2, indicating that the main sources of pollution were automobile exhaust, and the combustion of coal and biomass. The OC/EC minimum ratio method was used to estimate the secondary organic carbon (SOC) content in Beijing, Tianjin and Langfang. Their values were 10.73, 10.71, and 19.51, respectively, which accounted for 38%, 42%, and 37% of the average OC concentration in each city, respectively. The analysis of the eight carbon components showed that the main sources of pollutants in Beijing, Tianjin, and Langfang were exhaust emissions from gasoline vehicles, but the combustion of coal and biomass was relatively low. The pollution of road dust was more serious in Tianjin than in Beijing and Langfang. The contribution of biomass burning and coal-burning pollution sources to atmospheric carbon aerosols in Langfang was more prominent than that of Beijing and Tianjin.

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          Species Contributions to PM2.5 Mass Concentrations: Revisiting Common Assumptions for Estimating Organic Mass

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            Global warming in the twenty-first century: an alternative scenario.

            A common view is that the current global warming rate will continue or accelerate. But we argue that rapid warming in recent decades has been driven mainly by non-CO(2) greenhouse gases (GHGs), such as chlorofluorocarbons, CH(4), and N(2)O, not by the products of fossil fuel burning, CO(2) and aerosols, the positive and negative climate forcings of which are partially offsetting. The growth rate of non-CO(2) GHGs has declined in the past decade. If sources of CH(4) and O(3) precursors were reduced in the future, the change in climate forcing by non-CO(2) GHGs in the next 50 years could be near zero. Combined with a reduction of black carbon emissions and plausible success in slowing CO(2) emissions, this reduction of non-CO(2) GHGs could lead to a decline in the rate of global warming, reducing the danger of dramatic climate change. Such a focus on air pollution has practical benefits that unite the interests of developed and developing countries. However, assessment of ongoing and future climate change requires composition-specific long-term global monitoring of aerosol properties.
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              Identification of secondary organic aerosol episodes and quantitation of primary and secondary organic aerosol concentrations during SCAQS

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                Author and article information

                Journal
                Int J Environ Res Public Health
                Int J Environ Res Public Health
                ijerph
                International Journal of Environmental Research and Public Health
                MDPI
                1661-7827
                1660-4601
                13 July 2018
                July 2018
                : 15
                : 7
                : 1483
                Affiliations
                [1 ]Beijing Key Laboratory of Resources Environment and Geographic Information System, Capital Normal University, Beijing 100048, China; 2160902114@ 123456cnu.edu.cn (M.Q.); 2160902137@ 123456cnu.edu.cn (Y.L.); 2140901012@ 123456cnu.edu.cn (Q.X.); 2140902114@ 123456cnu.edu.cn (C.S.); 2160902100@ 123456cnu.edu.cn (X.L.); 2160902148@ 123456cnu.edu.cn (X.Y.)
                [2 ]Base of the State Key Laboratory of Urban Environmental Process and Digital Modelling, Beijing 100048, China
                [3 ]Beijing Municipal Research Institute of Environmental Protection, Beijing 100037, China; jiangle3657@ 123456sina.com
                Author notes
                [* ]Correspondence: 4973@ 123456cnu.edu.cn ; Tel.: +86-138-1070-7928
                Article
                ijerph-15-01483
                10.3390/ijerph15071483
                6069050
                30011803
                ca86eb3e-eb95-4407-a96a-6a0cbc518299
                © 2018 by the authors.

                Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license ( http://creativecommons.org/licenses/by/4.0/).

                History
                : 02 June 2018
                : 08 July 2018
                Categories
                Article

                Public health
                carbonaceous aerosols,pm2.5,organic carbon,elemental carbon,source analyses
                Public health
                carbonaceous aerosols, pm2.5, organic carbon, elemental carbon, source analyses

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